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PMEL Programs and Plans
Accomplishments in FY 97 and Plans for FY 98

Atmospheric Chemistry Project

Figures (a) Climatic effects of tropospheric aerosol, and (b) locatons of PMEL aerosol field studies.


Atmospheric Chemistry Program

Accomplishments in FY 97

The Atmospheric Chemistry Program at PMEL currently focuses on atmospheric aerosols and climate forcing. The Aerosol Project is designed to quantify the spatial and temporal distribution of natural and anthropogenic aerosols in the marine atmosphere and to determine the physical, meteorological and biogeochemical processes controlling their formation, evolution and properties. These data are needed in order (i) to aid the detection and attribution of regional and global climate change, in particular, the estimation of the alteration that anthropogenic aerosols may be providing to the greenhouse-gas induced warming patterns, and (ii) to improve the prediction of future climate changes for various radiative forcing scenarios.

The measurements made by PMEL during the first Aerosol Characterization Experiment (ACE-1) of the International Global Atmospheric Chemistry Project (IGAC) provided a means to characterize aerosol properties and assess the processes controlling the aerosol distribution in the lower marine boundary layer of the minimally polluted background marine atmosphere. The PMEL ACE-1 data analysis was completed in FY 97 and will be part of the ACE-1 Special Section of the Journal of Geophysical Research scheduled for publication in the summer of 1998.

The second activity of the PMEL Aerosol Project during FY 97 was our participation in ACE-2. PMEL took a lead role in this international IGAC aerosol experiment and coordinated the shipboard studies. ACE-2 was designed to study the radiative effects and controlling processes of anthropogenic aerosols from Europe and desert dust from the Africa as they are transported over the North Atlantic Ocean. The experiment involved over 250 research scientists from Europe and the United States and included 60 coordinated aircraft missions with 6 aircraft, one ship, and ground stations on Tenerife, Portugal and Madeira.

Another activity of the PMEL Aerosol Project is the chemical sampling and analysis of daily samples from a ground-based aerosol monitoring network. This network has been established in conjunction with NOAA/Climate Monitoring and Diagnostics Laboratory (CMDL) to determine means, variability, and possible trends of key optical, chemical and microphysical properties for a number of important aerosol types.


Atmospheric Chemistry Program

Plans for FY 98

  • Continue long-term aerosol monitoring with ion chromatographic and gravimetric analysis of daily submicron and weekly supermicron aerosol samples from the NOAA Aerosol Monitoring Network stations at Sable Island, Bondville, and Barrow.
  • Continue the development of a coupled aerosol chemical and optical model.
  • Complete data analysis and manuscripts describing region of high aerosol backscatter in the central equatorial North Pacific.
  • Complete manuscript describing aerosol chemical composition (what fraction is not sulfate) for marine, perturbed marine, clean continental, and polluted continental air masses.
  • Analyze data from ACE-2 and attend ACE-2 data workshops.
  • Begin organizing ACE-Asia. (Planning meetings in Nagoya, Japan, November 1997; Seattle, August 1998; white paper to be published in summer 1998.)

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